Question 6.6.Q1: For a given atomic number Z of the stopping medium, kinetic ......

For a given atomic number Z of the stopping medium, kinetic energy EKE_K of the light CP (electron or positron) at which both components of StotS_{tot} are identical is referred to as the critical kinetic energy EKcritE^{crit}_K . Radiation physics literature suggests that EKcritE^{crit}_K for a given stopping material Z can be estimated from the following empirical expression

EKcrit= const Z=800 MeVZE_{\mathrm{K}}^{\mathrm{crit}}=\frac{\text { const }}{Z}=\frac{800  \mathrm{MeV}}{Z}      (6.102)

(a) Fig. 6.14 plots Srad and ScolS_{rad}\ and\ S_{col} for seven stopping materials: helium, carbon, aluminum, copper, silver, lead, and uranium against the kinetic energy EKE_K of the light CP. Data are from the NIST and the plot is for EKE_K in the vicinity of EKcritE^{crit}_K for the seven stopping materials. Curves in Fig. 6.14 are not labeled. Identify Srad and ScolS_{rad}\ and\ S_{col} curves for the 7 stopping materials.

(b) From appropriately labeled Fig. 6.14 determine the critical kinetic energy EKcritE^{crit}_K of the 7 stopping materials, plot EKcritE^{crit}_K against Z and compare with a plot of (6.102). Discuss how (6.102) is satisfied for the 7 elements and draw general conclusions on the validity of (6.102) for stopping materials in general.

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(a) We identify the stopping power curves of Fig. 6.14 through accounting for the following two facts related to stopping powers of light CPs:

(1) For all stopping materials irrespective of atomic number Z the collision component ScolS_{col} of StotS_{tot} predominates at kinetic energies EKE_K < 10 MeV, while the radiation component SradS_{rad} of StotS_{tot} predominates at EKE_K > 100 MeV. In the intermediate region, where EKE_K is between 10 MeV and 100 MeV, the region of predominance depends on the atomic number Z of the stopping medium. Based on this we conclude that the heavy curves in Fig. 6.14 represent ScolS_{col} of the 7 stopping media and the light curves represent SradS_{rad} of the 7 stopping media (see Fig. 6.15).

(2) At a given kinetic energy EKE_K of the light CP, ScolS_{col} is inversely proportional to Z of the stopping medium as a result of two properties of the stopping medium: electron density Ne=ZNA/AN_e = ZN_A/A and mean ionization/excitation potential I , as evident from (6.17). Both NeN_e and ln I decrease ScolS_{col} with increasing Z. On the other hand, as shown in (6.3), SradS_{rad} is proportional to ZNeZN_e which suggests a linear proportion of SradS_{rad} with Z, since Z/A in Ne is essentially constant for all stopping media.

Scol=4πNe(e24πε0)2z2mec2β2{ln2mec2I+lnβ21 − β2β2CZδ}S_{\text{col}} = 4πN_e\left(\frac{e^2}{4πε_0}\right)^2\frac{z^2}{m_ec^2β^2}\left\{\ln\frac{2m_ec^2}{I}+\ln\frac{β^2}{1  −  β^2}−β^2 − \frac{C}{Z}− δ\right\} 

=C1Nez2β2Bˉcol.= C_1\frac{N_ez^2}{β^2}\bar{B}_{\text{col}}.           (6.17)

 

Srad=αre2ZNe(EK+mec2)Brad,S_{\text{rad}} = αr^2_eZN_e(E_K +m_ec^2)B_{\text{rad}}, (6.3)

In Fig. 6.14 we thus arrange the ScolS_{col} curves in the order of increasing Z from top (He) to bottom (U) and the SradS_{rad} curves in reverse order with U on the top and He on the bottom, as shown in Fig. 6.15.

(b) We are now ready to determine critical kinetic energy EKcritE_{\mathrm{K}}^{\mathrm{crit}} for the seven materials using data from Fig. 6.15. EKcritE_{\mathrm{K}}^{\mathrm{crit}} is defined as the intercept between ScolS_{col} and SradS_{rad} curves for the given stopping material and we can now read EKcritE^{crit}_K directly from the graph. The results for the 7 stopping media are listed in Table 6.13 in row (3). Also listed in the table is atomic number Z of the stopping medium in row (2) as well as in row (6) the critical energy EKcritE^{crit}_K determined from (6.102).
The measured and calculated EKcritE^{crit}_K data are plotted in Fig. 6.16 against atomic number Z of the various stopping materials with data points and solid curve, respectively. The agreement between the two sets appears to be reasonable, suggesting that (6.102) is a good and simple empirical approximation for determination of EKcritE^{crit}_K .

However, a comparison between rows (3) and (5) of Table 6.13 suggests otherwise, especially for stopping media of low Z. We therefore re-plot the data in the form of EKcrit ×ZE_{\mathrm{K}}^{\text {crit }} \times Z and get a better picture on the discrepancy between (6.102) and the NIST data, as shown in Fig. 6.17. The grey area in the figure shows a region of ±10 % agreement with (6.102) and we note that for Z < 30 data calculated with (6.102) exceed the NIST data by more than 10 % and the discrepancy margin increases as Z decreases.
Figure 6.17 shows that (6.102) must be used with caution, especially at low atomic number Z where it overestimates the critical kinetic energy EKcritE_{\mathrm{K}}^{\mathrm{crit}} by ∼50 %. At large Z (6.102) provides a more reliable means for estimation of the critical kinetic energy EKcritE_{\mathrm{K}}^{\mathrm{crit}} achieving an accuracy of about ±5 %.

Table 6.13 Critical kinetic energy of various stopping media. Measured data are obtained from the NIST, calculated data are determined from (6.102)
 (1)  Stopping medium  Helium  He  Carbon C Alumin Al Copper Cu Silver Ag Lead Pb Uran U (2)  Atomic number Z261329478292 (3) EKcrit (MeV) measured  data 277965124.316109(5)EKcrit ×Z(MeV) measured  data 554576663705752820823(6)EKcrit (MeV) calculated  from (6.102)40013361.527.617.09.88.7(7)EKcrit ×Z(MeV) calculated from (6.102)800800800800800800800(8)Scol =Srad(MeVcm2/g)2.731.951.791.531.411.201.14\begin{array}{lllllllll} \hline \text { (1) } & \text { Stopping medium } & \begin{array}{l} \text { Helium } \\ \text { He } \end{array} & \begin{array}{l} \text { Carbon } \\ \mathrm{C} \end{array} & \begin{array}{l} \text { Alumin } \\ \mathrm{Al} \end{array} & \begin{array}{l} \text { Copper } \\ \mathrm{Cu} \end{array} & \begin{array}{l} \text { Silver } \\ \mathrm{Ag} \end{array} & \begin{array}{l} \text { Lead } \\ \mathrm{Pb} \end{array} & \begin{array}{l} \text { Uran } \\ \mathrm{U} \end{array} \\ \hline \text { (2) } & \text { Atomic number } Z & 2 & 6 & 13 & 29 & 47 & 82 & 92 \\ \hline \text { (3) } & \begin{array}{l} E_{\mathrm{K}}^{\text {crit }}(\mathrm{MeV}) \text { measured } \\ \text { data } \end{array} & 277 & 96 & 51 & 24.3 & 16 & 10 & 9 \\ \hline(5) & \begin{array}{l} E_{\mathrm{K}}^{\text {crit }} \times Z(\mathrm{MeV}) \text { measured } \\ \text { data } \end{array} & 554 & 576 & 663 & 705 & 752 & 820 & 823 \\ \hline(6) & \begin{array}{l} E_{\mathrm{K}}^{\text {crit }}(\mathrm{MeV}) \text { calculated } \\ \text { from }(6.102) \end{array} & 400 & 133 & 61.5 & 27.6 & 17.0 & 9.8 & 8.7 \\ \hline(7) & \begin{array}{l} E_{\mathrm{K}}^{\text {crit }} \times Z(\mathrm{MeV}) \\ \text { calculated from }(6.102) \end{array} & 800 & 800 & 800 & 800 & 800 & 800 & 800 \\ \hline(8) & \begin{array}{l} S_{\text {col }}=S_{\mathrm{rad}}\left(\mathrm{MeV} \cdot \mathrm{cm}^2 / \mathrm{g}\right) \end{array} & 2.73 & 1.95 & 1.79 & 1.53 & 1.41 & 1.20 & 1.14 \\ \hline \end{array}

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